The invention discloses a method for removing polycyclic aromatic hydrocarbons in a water body by using an iron-manganese bimetallic oxide modified biological carbon photo-Fenton composite material, which comprises the following steps: mixing the composite material with the water body containing the polycyclic aromatic hydrocarbons, stirring, adding hydrogen peroxide solution, and carrying out photo-Fenton reaction to complete the removal of polycyclic aromatic hydrocarbons in the water body, wherein the composite material comprises biochar and the iron-manganese bimetallic oxide attached to the biochar; the iron-manganese bimetallic oxide is a mixture of iron oxide and manganese oxide, wherein the iron oxide comprises Fe3O4 and Fe2O3, and the manganese oxide comprises Mn3O4 and Mn2O3. Themethod has the advantages of simple process, simple and convenient operation, low cost, high removal efficiency, good removal effect, wide application range, good recycling performance, environmentalfriendliness and the like, and the method can be widely adopted and can efficiently remove polycyclic aromatic hydrocarbons in the water body, and has high application value and commercial value.