The invention belongs to the field of inorganic nano structure materials, in particular to a method for inorganically synthesizing organized mesoporous alumina, which is characterized in that inorganic matters of sodium aluminate and aluminum chloride are in acid-base pairing to prepare mesoporous alumina which has large specific surface area, narrow pore-size distribution, organized pore channel and high hydrothermal stability; and methyl cellulose which is used as a template agent in a synthesizing process has thermosensitivity and is beneficial to recycle. The method for inorganically synthesizing organized mesoporous alumina has the characteristics that raw materials have low cost, the template agent can be recycled, the technology is simple and easy to control, and the like. The method for inorganically synthesizing organized mesoporous alumina is easy to realize industrial production, and the obtained organized mesoporous alumina has wide application prospect in the fields of catalytic reaction, adsorption, separation, and the like.