The invention discloses a diamond color center gyroscope based on Aharonov-Anandan geometric phase and an angular velocity measuring method. The gyroscope comprises a reflector, a permanent magnet, a substrate, a diamond sample, first microwave coils, second microwave coils, multiple area array CCDs, multiple filters, a third microwave coil, a first convex lens, a laser device, a polarizing sheet, a dichroscope and a second convex lens. The method for measuring angular velocity by means of the diamond color center gyroscope is further provided. The gyroscope has the advantages of being small in size, large in measuring range and the like, and therefore the gyroscope has potential application in producing ammunition.