The invention relates to a
graphene-based
dielectric elastomer composite material and a preparation method thereof. The
composite material comprises an
elastomer base body,
graphene oxide-based
dielectric filler and a cross-linking
system, wherein the
graphene oxide-based
dielectric filler is core-shell
hybrid particles of flaky graphene
oxide-coated
nano carbon balls. The method disclosed by the invention utilizes phi-phi
electron interaction and
hydrogen-bond interaction to realize simple and effective self-assembling of graphene oxide and
nano carbon balls, so that the core-shell
hybrid particles of the graphene oxide-coated
nano carbon balls are formed and then added into rubber
emulsion; then, an in-situ thermal reduction method is used for reducing a shell layer into graphene, so that a three-dimensional isolated
network structure of latex particles coated by core-shell
hybrid particles is formed, and therefore, dispersion of the graphene oxide is improved, dosage of the graphene and
elastic modulus of the
composite material are effectively lowered, and electro-generated deformation performances are remarkably improved; the high-performance graphene-based dielectric
elastomer composite material with great electro-generated deformation under low driving
voltage is prepared, and when
electric field strength is 2kV / mm, deformation amount can reach 3.06%.